From 2-methylimidazole to 1,2,3-triazole: a topological transformation of ZIF-8 and ZIF-67 by post-synthetic modification
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Date
2017
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ROYAL SOC CHEMISTRYTHOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND
Abstract
Bridging ligand replacement in zeolitic imidazolate frameworks, ZIF-8 and ZIF-67, by 1,2,3-triazole was investigated. A complete substitution of 2-methylimidazole by 1,2,3-triazole resulted in a topological transformation of the parent framework from a sodalite (SOD) network to a diamond (DIA) network.
Description
This work was supported by The Scientific and Technological Research Council of Turkey TUBITAK under the contract No. 214M397. For work at Northwestern, J. T. H. and O. K. F. and gratefully acknowledge support from the Dept. of Energy, Office of Science, Basic Energy Science through grant DE-FG02-08ER155967.
Keywords
METAL-ORGANIC FRAMEWORKS, ZEOLITIC IMIDAZOLATE FRAMEWORKS, ASSISTED LINKER EXCHANGE, DE-NOVO SYNTHESIS
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Volume 53 Issue 12 Page 2028-2031