WoS İndeksli Yayınlar Koleksiyonu
Permanent URI for this collectionhttps://hdl.handle.net/20.500.12573/394
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Article Colloidal Photodetectors Based on Engineered Multishelled InP Based Quantum Dots(Institute of Physics, 2026-01-08) Akrema; Erol, E.; Savaş, M.; Yazici, A.; Erdem, T.; Mutlugün, E.; Faruk Yazıcı, AhmetIn this work, we present a straightforward and cost-effective approach to synthesize multi-shell InP/ZnSe/ZnSeS/ZnS quantum dots (QDs) that show promising potential for use in photodetectors. By carefully layering ZnSe, ZnSeS, and ZnS shells around an InP core, we were able to enhance the stability and optical performance of the QDs, achieving a narrow emission peak of 45 nm and a high photoluminescence quantum yield of 55%. These QDs were then integrated into simple photodetector devices, which possessed impressive sensitivity and detection capabilities. Specifically, our devices achieved a peak responsivity of 0.54 A W−1 and a detectivity of 2.22 × 1011 Jones at 400 nm with a 5 V bias. This study highlights the potential of InP-based QDs as a safer and more sustainable alternative to traditional QDs that contain toxic heavy metals, offering a viable path forward for developing high-performance optoelectronic devices. Our findings suggest that these InP/ZnSe/ZnSeS/ZnS QDs could be a key material for the next generation of high-performance optoelectronic devices, especially in applications that require highly sensitive and stable photodetectors. © 2026 The Author(s). Published by IOP Publishing Ltd.Article Citation - WoS: 4Citation - Scopus: 3Multifaceted Effects of the Dielectric Component Within Plasmon-Assisted Light-Emitting Structures(American Chemical Society, 2025-10-23) Kulakovich, O.; Muravitskaya, A.; Ramanenka, A.; Efimova, T.; Krukov, V.; Mutlugün, E.; Gaponenko, S.Plasmon-enhanced photoluminescence of molecular probes and semiconductor nanocrystals is a rapidly developing field that promises enhanced sensitivity in chemical and biomedical analyses, as well as higher efficiency of light-emitting devices and single-photon sources. The dielectric component, or spacer, is typically used to control the distance between the emitter and the plasmonic nanoparticle in order to decrease undesirable nonradiative energy transfer to the metal and achieve high enhancement efficiency. While most research focuses on the shape and organization of the plasmonic nanoparticles, less attention is given to the role of the dielectric component in plasmon-enhancing structures. Meanwhile, the dielectric shell or environment critically modulates near-field enhancement, far-field scattering, charge and energy exchange between the emitter and the plasmonic structure, and the general environmental stability of the structure. In this review, we discuss all mentioned topics and therefore consider both the optical and chemical influence of the widely used spacers and dielectric layers on plasmon-enhanced photoluminescence efficiency. Investigating the role of individual components in plasmon-assisted light-emitting structures is critical for optimizing device performance and for advancing the integration of plasmonic architectures in optoelectronic and sensing applications. This review challenges the passive interpretation of dielectrics, revealing them as one of the key players in plasmonic structures, mediating field enhancement, emission dynamics, and chemical stability simultaneously. © 2025 American Chemical Society