Browsing by Author "Onses, Mustafa Serdar"

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Inkjet Printing of Aqueous Silver Inks on Water-Soluble Fabrics for Transient Electronics Applications
(AMER CHEMICAL SOC, 2024) Gozutok-Onses, Zehra; Kiremitler, N. Burak; Ozbasaran, Aleyna; Huang, Xian; Onses, Mustafa Serdar; Usta, Hakan; 0000-0002-0618-1979; AGÜ, Mühendislik Fakültesi, Malzeme Bilimi ve Nanoteknoloji Mühendisliği Bölümü; Gozutok-Onses, Zehra; Usta, Hakan
There is an urgent need to develop practical routes for manufacturing transient electronic devices to tackle the emerging issue of electronic waste and enable next-generation devices. This study reports additive patterning of conductive layers on industrially available water-soluble nonwoven fabrics composed of poly(vinyl alcohol) (PVA). Aqueous inks composed of reactive silver precursors can be practically patterned over water-soluble fabrics by inkjet printing. The efficient deposition of materials with droplet volumes on the order of picoliters ensures the generation of conductive patterns on a water-soluble fabric using a solution-processable fabrication with aqueous inks. The fabrication of conductive electrodes and transience behavior are studied on PVA fabrics with two different degrees of hydrolysis, providing tunability in the temperature-dependent degradation of the substrate. The application of the printed conductive pads is demonstrated in resistive heaters. The temperature of the fabric can exceed 100 degrees C in less than 15 s at a safe voltage of 3 V. The heater exhibits stable operation under cyclic heating and cooling. The presented approach presents key opportunities in additive patterning of aqueous solutions and colloidal dispersions over water-soluble substrates for transient device applications.
Structurally Colored Physically Unclonable Functions with Ultra-Rich and Stable Encoding Capacity
(WILEY-Advanced, 2025) Esidir, Abidin; Ren, Miaoning; Pekdemir, Sami; Kalay, Mustafa; Kayaci, Nilgun; Gunaltay, Nail; Usta, Hakan; Huang, Xian; Onses, Mustafa Serdar; 0000-0002-0618-1979; AGÜ, Mühendislik Fakültesi, Malzeme Bilimi ve Nanoteknoloji Mühendisliği Bölümü; Usta, Hakan
Identity security and counterfeiting assume a critical importance in the digitized world. An effective approach to addressing these issues is the use of physically unclonable functions (PUFs). The overarching challenge is a simultaneous combination of extremely high encoding capacity, stable operation, practical fabrication, and a widely available readout mechanism. Herein this challenge is addressed by designing an optical PUF via exploiting the thickness-dependent structural color formation in nanoscopic films of ZnO. The structural coloration ensures authentication using widely available bright-field-based optical readout, whereas the metal oxide provides a high degree of structural stability. True physical randomness in spatial position is achieved by physical vapor deposition of ZnO through stencil masks that are fabricated by pore formation in polycarbonate membranes via photothermal processing of stochastically positioned plasmonic nanoparticles. Structural coloration emerges from thin film interference as confirmed via simulation studies. The rich color variation and stochastic definition of domain size and geometry result in chaotic features with an encoding capacity that approaches (6.4 x 105)(2752x2208). Deep learning-based authentication is further demonstrated by transforming these chaotic features into unbreakable codes without field limitations. This ultra-rich encoding capacity, coupled with outstanding thermal and chemical stability, forms a new cutting edge for state-of-the-art PUF-based encoding systems.